Peer-reviewed

Leaf-made zinc oxide nanoparticles show strong corrosion inhibition

In laboratory tests on carbon steel in 1 M hydrochloric acid, both routes showed high reported inhibition at 100 ppm, but they ranked differently across electrochemical tests.

Zinc oxide nanoparticles made with Bauhinia purpurea leaf extract showed high reported corrosion inhibition in a laboratory comparison of two synthesis routes. At 100 parts per million (ppm), the sol-gel condition had a reported inhibition efficiency of 97.7% in potentiodynamic polarization (PDP), compared with 94.1% for co-precipitation. PDP is the electrochemical test used here to report corrosion current density and inhibition efficiency. The route ranking changed in electrochemical impedance spectroscopy (EIS), a separate electrochemical readout: co-precipitation was reported at 99% inhibition and sol-gel at 98%.

The PDP current-density readings matched that ordering: 50 µA cm−2 for co-precipitation and 19.4 µA cm−2 for sol-gel at 100 ppm. Current density is the corrosion-related electrical signal reported for the coupon, so the lower sol-gel value was consistent with its higher PDP inhibition percentage. The close but opposing results make the route comparison more nuanced than a simple overall ranking.

A narrow laboratory comparison

The experiment used cylindrical carbon-steel coupons with a reported surface area of 1 cm² and a diameter of 10 mm. The researchers compared zinc oxide nanoparticles made by co-precipitation and sol-gel synthesis. The formulations were tested in 1 M hydrochloric acid at 50, 75 and 100 ppm. Those details define the setting in which the inhibition figures were obtained.

The electrochemical work used a three-electrode cell. The protocol recorded open-circuit potential before PDP and performed EIS at open-circuit potential, with repeated EIS experiments averaged. Alongside those measurements, the reported characterization included Fourier-transform infrared spectroscopy (FTIR), ultraviolet-visible spectroscopy (UV-vis), scanning electron microscopy and energy-dispersive spectroscopy (SEM/EDS), and X-ray photoelectron spectroscopy (XPS). In ordinary terms, the electrochemical tests supplied the corrosion-inhibition readings, while the other methods examined the nanoparticles and surfaces.

Dissolved iron fell in the inhibitor tests

A separate chemical measurement pointed in the same direction. Atomic absorption spectroscopy (AAS) reported 3.45 mg L−1 of dissolved iron in the blank condition. At 100 ppm, the reported dissolved-iron concentration was 0.83 mg L−1 for co-precipitation and 0.73 mg L−1 for sol-gel. Both inhibitor conditions were therefore associated with less iron in solution than the blank, with sol-gel showing the lower of the two treated values.

What the measurements can support

The authors interpret the electrochemical, iron-dissolution and surface findings as consistent with adsorption of leaf phytochemicals and zinc oxide nanoparticles onto the steel. In that interpretation, the adsorbed material forms a protective organic-inorganic film. They classify the inhibitor as mixed-type and report Langmuir adsorption behavior, based on the way the data fit that model. These are the authors' explanations of the combined measurements; the reported tests do not by themselves establish a definitive molecular mechanism or a universal route winner.

The reach of the result is narrower than the percentages may suggest. The evidence is limited to laboratory carbon-steel coupon tests in 1 M HCl, using the three reported nanoparticle concentrations. It does not show how stable the proposed film would be during long-term practical service, whether the route ranking would persist with other steel grades or acid conditions, or whether the material is environmentally safe, biodegradable, non-toxic or cheaper. No human, animal or field-structure evidence is part of this study.

For materials researchers, the result is best read as a laboratory proof of concept: under the tested setup, the leaf-mediated ZnO nanoparticles were associated with high electrochemical inhibition readings and lower dissolved-iron readings than the blank. Broader testing would need to check other steels, acid conditions and longer exposures, as well as whether the route-dependent pattern persists. Until then, co-precipitation and sol-gel both show strong reported performance under the specified conditions, but the two electrochemical tests do not produce a definitive overall route winner.

Paper data and sources

Original title: Corrosion inhibition evaluation of Bauhinia purpurea extract mediated ZnO nanoparticles for carbon steel in acidic environment.
Authors: O Swathy, S Shanmuga Priya, Meghana K Navada, Lavanya Mulky
Journal/Repository: Discover nano
Status: Peer-reviewed
First online: 2026-08-21
DOI: 10.1186/s11671-026-04826-w
Original paper · Full text

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